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A radiofrequency heated reactor system for post-combustion carbon capture

机译:用于燃烧后碳捕集的射频加热反应器系统

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摘要

Several problems with stabilization of electricity grid system are related to the time lag between the electricity supply and demand of the end users. Many power plants run for a limited period of time to compensate for increased electricity demand during peak hours. The amount of CO2 generated by these power installations can be substantially reduced via the development of new demand side management strategies utilizing CO2 absorption units with a short start-up time. The sorbent can be discharged using radiofrequency (RF) heating to fill the night-time valley in electricity demand helping in the stabilization of electricity grid. Herein a concept of RF heated fixed bed reactor has been demonstrated to remove CO2 from a flue gas using a CaCO3 sorbent. A very stable and reproducible operation has been observed over twenty absorption-desorption cycles. The application of RF heating significantly reduced the transition time required for temperature excursions between the absorption and desorption cycles. The effect of flow reversal during desorption on desorption time has been investigated. The desorption time was reduced by 1.5 times in the revered flow mode and the total duration of a single absorption-desorption cycle was reduced by 20%. A reactor model describing the reduced desorption time has been developed.
机译:电网系统稳定的几个问题与最终用户的电力供需之间的时滞有关。许多发电厂仅在有限的时间内运行以补偿高峰时段的用电需求。通过开发新的需求侧管理策略,利用短时间内启动的CO2吸收单元,可以大大减少这些电力设备产生的CO2量。可以使用射频(RF)加热来释放吸附剂,以填补电力需求的夜间谷底,从而有助于稳定电网。在本文中,已经证明了RF加热的固定床反应器的概念使用CaCO 3吸附剂从烟道气中去除CO 2。在二十个吸收-解吸循环中,观察到非常稳定且可重复的操作。射频加热的应用大大缩短了吸收和解吸循环之间温度漂移所需的过渡时间。研究了解吸过程中逆流对解吸时间的影响。在逆流模式下,解吸时间减少了1.5倍,单个吸收-解吸循环的总持续时间减少了20%。已经开发出描述减少的解吸时间的反应器模型。

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